Development and performance evaluation of flow-electrode capacitive deionization (FCDI) module featuring spiral-wounded (SW) structures

AuthorHendrajaya, Glenn Lucas
Call NumberAIT Thesis no.EV-26-02
Subject(s)Saline water conversion
NoteA thesis submitted in partial fulfillment of the requirements for the degree of Master of Engineering in Environmental Engineering and Management
PublisherAsian Institute of Technology
AbstractFlow-electrode capacitive deionization (FCDI) offers significant advantages in continuous desalination; however, conventional plate-and-frame modules face limitations in scalability and packing density. This research introduces a novel Spiral-Wound FCDI (SWFCDI) architecture, developed through three iterative generations (V1, V2, and V3) to optimize hydraulic distribution and spatial efficiency. The V1 prototype identified critical design drawbacks, including geometric imbalances between membrane lengths and high pumping resistance. These were addressed in the V2 and V3 designs by integrating a dual-channel configuration and an upgraded 5-hole multi-port distribution system to ensure uniform slurry dispersion. Experimental evaluation was conducted under a constant voltage of 1.4 V, using a 10% (w/v) carbon loading and a 5 g/L NaCl feed. Results demonstrated that the architectural upgrades successfully expanded the effective area (Aeff) from 45 cm² to 105 cm², achieving a superior packing density of 0.523 cm⁻¹ that has 7 to 12-fold improvement over traditional plate-and-frame modules. While V1 exhibited a high initial Average Salt Removal Rate (ASRR) of 1.092 μmol/cm²/min, the optimized V3 module was the only configuration to achieve complete desalination (>99.23% SRE) within 160 minutes. Despite these performance gains, the study identified a trade-off in energy efficiency; the Coulombic Efficiency (CE) ranged from 77.7% to 84.8%, primarily due to carbon clogging induced by the internal spacer mesh. Consequently, the specific energy consumption (Ev) reached 3.98 kWh/m³ for total salt removal. These findings establish the SWFCDI as a highly compact and potent platform for high-purity water production, while highlighting the necessity for slurry optimized spacers in future iterations to bridge the gap between laboratory-scale prototypes and practical industrial implementation.
Year2026
TypeThesis
SchoolFaculty of Civil and Environmental Engineering (2026)
DepartmentOther Field of Studies (No Department)
Academic Program/FoSEnvironmental Engineering and Management (EEM)
Chairperson(s)Xue, Wenchao
Examination Committee(s)Thammarat Koottatep;Ghimire, Anish
Scholarship Donor(s)Global Water & Sanitation Center (GWSC);AIT Scholarship
DegreeThesis (M. Eng.) - Asian Institute of Technology, 2026


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